He is a religious zealot, his immortality came from the Jashin faith experiments. We do not know whether Jashin is "real" and whether the immortality only works while he is a Jashin zealot or if his abilities came from "just experiment".
If it is not actually faith connected, then yes, he could in theory also gain a calm mind and find tactics that are more suitable to his abilities, for example, infiltration and stealth--just get some blood as stealthy as possible, run away, do the ritual, it's game over.
But if any part of his ability actually came from the religious zeal itself, then it won't work, because any of that directly contradicts with the faith and doesn't qualify as "zeal" in any faith.